|  
  
  Growing of hexagonal compact domains in a granular compaction experiment. 
Watch the movie
  
  Flowing of metallic balls in a rotating drum
  
  Vibrated granular layer. Watch the movie
  
  
 | About me
By chance my professional activities are combining my passions for sciences and technologies. 
I’m using extensively competencies in electronics, programming, and mechanics to develop original 
measurement devices for research projects and to illustrate my lectures. These competencies were 
mainly developed in the framework of my hobbies: DIY electronics, 
aeromodelling, mechanics, blacksmithing and bladesmithing.
 PositionLectures
Some pictures of the experiments performed to illustrate my lectures:General Physics (for students in pharmacy)Thermodynamics (for bio-engineers)Waves and Quanta (for engineers)Techniques of Experimental Physics (for students in physics)Numerical tools for Soft Matter Physics (for students in physics) 
        
     ResearchSoft matter  -
Cohesive granular materials -
Static, quasistatic and dynamical properties of granular materials -
Effect of a magnetic and electric field on a granular material -
Powder electrostatics -
Self Assembly processes -
Active materials -
Colloids
 
 Research strategy - Our strategy to study a physical phenomenon is based on the development of original experimental set-ups to obtain original experimental results. Afterward, physical models are proposed to describe the physical mechanisms and to extract the main parameters. If needed, numerical simulations are conducted to investigate parameters which are difficult to control experimentally. Sometimes, laboratory prototypes developed to perform fundamental studies are becoming commercial instruments.     Physics of powders and granular materials. - A granular material is a conglomeration of discrete solid particles. Granular materials behavior is influenced by (1) steric repulsions, (2) friction forces (3) cohesive forces and (4) interaction with the surrounding gas. The steric repulsion is related to the grain geometry. Friction forces are influenced by both the surface state (rough or smooth surface) and the chemical nature of the grains. Cohesive forces may be induced by the presence of liquid bridges, by electrostatic charges, by van der Waals interactions or more rarely by magnetic dipole-dipole interactions. The predominance of one of these forces depends on both the environmental conditions and the physico-chemical properties of the grains. When the weight of one grain is higher than the cohesive forces, the material is considered as non-cohesive. These materials have been intensively studied during the last decades because of the rich variety of their physical properties. On the other hand, if the cohesive forces acting on a grain are higher than the weight of the grain, these cohesive forces will drastically modify the properties of the pile. Among these cohesive granular materials, fine powders are used in many research domains : chemistry, pharmacy, engineering... Nowadays, the processes used for the manipulation of powders are still mainly based on empirical knowledge. However, the complexity of the methods used in these domains induces the necessity of more rigorous knowledge of these materials. Therefore, fundamental studies of cohesive powders are still essential.     Model cohesive powders. - The difficulty to quantify and to control cohesion between the grains of a powder makes their experimental study very complex. Therefore, we first used a controlled cohesive powder made of metallic grains in an adjustable magnetic field B [18, 21]. In this controlled system, the cohesion between the grains can the tuned easily through the magnetic field. This system has been used during to study the influence of the cohesion on packing fraction, repose angle, heap shape, flow in silos and on the flow in a rotating drum.   Real cohesive powders. - After the study of model cohesive powders with a fundamental approach, we analyzed (and are still analyzing) the behavior of powders used in the industry with a more practical approach [25]. For that, we developped a range of original set-ups to measure packing dynamics, powder rheology, powder electrostatic properties, cohesiveness,... At the beginning, these set-ups were laboratory prototypes. After repetitive expressions of interest from industries, these methods were adapted to become commercial laboratory instruments:
GranuFlow,
GranuPack,
GranuDrum,
GranuHeap,
GranuMidity
and GranuCharge. These instruments are now commercialized by the company GranuTools. Combined effect of humidity and electrostatic charges on powders. - When two materials are rubbed, electric charges are exchanged at the surfaces. This contact electrification is an old fundamental scientific subject. However, despite the numerous studies dedicated to this subject, the fundamental mechanisms behind the triboelectric effect are not fully understood in powders and granular materials. The electric charges created by triboelectric effects lead to uncontrolled electric field, electrostatic forces between the grains and/or between the grains and the container. Moisture is known to affect both static and dynamic behaviors of granular materials. Moreover, the effect of moisture is far from obvious due to the interplay with electrostatic effects. Indeed, moisture influences both surface grains conductivity and capillary bridges formation. For low relative air humidity, the electrical conductivity necessary for charge dissipation is reduced. For high relative air humidity, the electrical conductivity increases and liquid bridges may be formed at the contacts between the grains, resulting in sticking. Therefore, the electrical charges are dissipated more easily. However, the apparition of liquid bridges also induces cohesive forces inside the packing. At intermediate relative humidity values the cohesion is expected to be lower. We performed different studies on that topic. In particular, we analyzed the effect of powder flow aid additives (fumed silica, mesoporous silica, stearate, ...) on these cohesive forces.
   Self assembly processes - My present research project includes a second axis dedicated to the study of self-assembly processes leading to the formation of mesostructures. Mesostructures are microscopic (typically from 100 nanometers to 100 microns) architectures with complex arrangements which confer them remarkable physical properties. Static and dynamic properties of such structures are investigated using model systems of Soft Matter. This activity is based on expertise acquired during my experimental works on collective motions, and patterning in granular materials. These self-organization processes take place in assemblies of micro and nano particles placed in an external field (magnetic and/or electric) and submitted to geometrical, mechanical, capillary and hydrodynamic constraints. In order to identify and to control the relevant self-assembly processes, the interactions between the particles have to be studied precisely. With a better fundamental understanding of these interactions, the self-organization processes will be obtained through a bottom-up method instead of the classical empirical methods. Then, we will be able to improve the long-range organization in mesostructures, catalyst, porous materials, sintered materials, ... Moreover, future studies will be dedicated to reversible self-organized systems where the order could be modified in order to obtain smart reconfigurable materials.
 Publications1. Compaction of anisotropic granular materials: Experiments and simulationsPhys. Rev. E
70, 051314
 (2004)
 Show Abstract
 
 2. Grain mobility and hexagonal domains formation in 2d granular compaction
 Powders & Grains
1, 343
 (2005)
 Show Abstract
 
 
 | 3. Experimental Study of Granular Compaction Dynamics at Different Scales: Grain Mobility, Hexagonal Domains, and Packing Fraction Phys. Rev. Lett.
95, 028002
 (2005)
 Show Abstract
 
 |  | 
|---|
 4. Experimental study of the compaction dynamics for two-dimensional anisotropic granular materials
 Phys. Rev. E
74, 021301
 (2006)
 Show Abstract
 
 5. Compaction of granular materials: experiments and contact dynamics simulations
 J. Phys.: Conf. Ser.
40, 133
 (2006)
 Show Abstract
 
 6. Linking compaction dynamics to the flow properties of powders
 Appl. Phys. Lett.
89, 093505
 (2006)
 Show Abstract
 
 7. Precursors to avalanches in a granular monolayer
 Phys. Rev. E
74, 031311
 (2006)
 Show Abstract
 
 8. The influence of grain shape, friction and cohesion on granular compaction dynamics
 Eur. Phys. J. E
22, 241
 (2007)
 Show Abstract
 
 9. Kinetic Energy Fluctuations and Diffusivity in a 2D Vibrated Granular Packing
 TRAFFIC AND GRANULAR FLOW 2007
, 597
 (2007)
 Show Abstract
 
 10. TUNABLE RANDOM PACKINGS
 New J. of Phys.
9, 406
 (2007)
 Show Abstract
 
 
 | 11. Swarming and swirling in self-propelled polar granular rods Phys. Rev. Lett.
100, 058001
 (2008)
 Show Abstract
 
 |  | 
|---|
 12. Stationary states in 1D system of inelastic particles
 Ukr. Journ. Phys. 
53, 1128
 (2008)
 Show Abstract
 
 13. Controlled flow of Smart Powders
 Phys. Rev. E
78, 061302
 (2008)
 Show Abstract
 
 14. Mullite coatings on ceramic substrates: stabilisation of Al2O3-SiO2 suspensions for spray drying of composite granules suitable for reactive plasma spray
 J. of Eur. ceramic soc.
29, 2169
 (2008)
 Show Abstract
 
 15. Motion of carbon nanotubes in a rotating drum: The dynamic angle of repose and a bed behavior diagram
 Chem. Eng. J.
146, 143
 (2009)
 Show Abstract
 
 16. Packing fraction and compaction dynamics of magnetic powders
 AIP Conf. Proc.
1145, 131-134
 (2009)
 Show Abstract
 
 17. Flow properties and heap shape of magnetic powders
 AIP Conf. Proc.
1145, 135-138
 (2009)
 N. Vandewalle & G. Lumay
 The flow properties of powders are mainly related to the interplay of cohesive forces and intergrain frictional forces. Indeed, the formation of large aggregates and the presence of arches modify the dynamic and the static properties of a powder. We have experimentally investigated a "smart powder" for which the interparticle interaction can be tuned by an external magnetic field. Through our experimental results, we show that the rheological and the static properties of such a system can be controlled. (i) Different dynamical flowing regimes have been observed through the output of  funnel like a "dry liquid state" forming conic droplets as well as a "layered soft state". (ii) The morphology of a cohesive heap have been also analyzed. The increase of the heap height h with the applied magnetic field strength has been measured for different orientations of the field. Moreover, a strong anisotropy of the heap shape is observed when the magnetic field is oriented perpendicularly to the gravity.
 Hide Abstract
 
 18. Compaction dynamics of a magnetized powder
 Phys. Rev. E
80, 041302
 (2009)
 Show Abstract
 
 19. Effect of an electric field on an intermittent granular flow
 Phys. Rev. E
81, 041309
 (2010)
 Show Abstract
 
 20. Compaction dynamics of wet granular assemblies
 Phys. Rev. Lett.
105, 048001
 (2010)
 Show Abstract
 
 21. Flow of magnetized grains in a rotating drum
 Phys. Rev. E
82, 040301(R)
 (2010)
 Show Abstract
 
 22. A pendulum test as a tool to evaluate viscous friction parameters in the equine fetlock joint
 The Veterinary Journal
188, 204
 (2011)
 Show Abstract
 
 23. Influence of a reduced gravity on the volume fraction of a monolayer of spherical grains
 Phys. Rev. E
84, 041305
 (2011)
 Show Abstract
 
 24. Granular gas in a periodic lattice
 Eur. Phys. J. E
32, 1465
 (2011)
 Show Abstract
 
 25. Measuring the flowing properties of powders and grains
 Powder Technology
224, 19
 (2012)
 Show Abstract
 
 26. How relative humidity affects random packing experiments
 Phys. Rev. E
85, 031309
 (2012)
 Show Abstract
 
 27. Hysteretic behavior in three-dimensional soap film rearrangements
 Phys. Rev. E 
83, 021403
 (2011)
 Show Abstract
 
 28. Symmetry breaking in a few-body system with magnetocapillary interactions
 Phys. Rev. E 
85, 041402
 (2012)
 Show Abstract
 
 29. Cascade of flows for characterizing segregation of granular mixtures
 Powder Technology
234, 32
 (2013)
 Show Abstract
 
 30. Breaking arches with vibrations: the role of defects and friction
 Phys. Rev. Lett. 
109, 068001
 (2012)
 Show Abstract
 
 31. Flow abilities of powders and granular materials evidenced from dynamical tap density measurement
 Powder Technology
235, 842
 (2013)
 Show Abstract
 
 32. Experimental study of a vertical column of grains submitted to a series of impulses
 European Physical Journal E
36, 16
 (2013)
 Show Abstract
 
 33. Influence of the gravity on the discharge of a silo
 Granular Matter 
15, 263
 (2013)
 Show Abstract
 
 . Self-assembled magnetocapillary swimmers
 Soft Matter
9, 2420
 (2013)
 Show Abstract
 
 35. Melting of a confined monolayer of magnetized beads
 Phys. Rev. E 
87, 062201
 (2013)
 Show Abstract
 
 36. Mesoscale structures from magnetocapillary self-assembly
 Eur. Phys. J. E
36, 127
 (2013)
 Show Abstract
 
 37. Customizing mesoscale self-assembly with three-dimensional printing
 New J. of Phys.
16, 023013
 (2014)
 Show Abstract
 
 38. Quantitatively mimicking wet colloidal suspensions with dry granular media
 Scientific reports
5, 10348
 (2015)
 Show Abstract
 
 39. Bernal random loose packing through freeze-thaw cycling
 Phys. Rev. E
92, 010202
 (2015)
 Show Abstract
 
 40. Rheological behavior of β-Ti and NiTi powders produced by atomization for SLM production of open porous orthopedic implants
 Powder Technology
283, 199
 (2015)
 Show Abstract
 
 41. Linking flowability and granulometry of lactose powders
 International Journal of Pharmaceutics
494, 312
 (2015)
 Show Abstract
 
 . Remote control of self-assembled microswimmers
 Scientific reports
5, 16035
 (2015)
 Show Abstract
 
 43. Flow of magnetic repelling grains in a two-dimensional silo
 Papers in Physics
7, 070013
 (2015)
 Show Abstract
 
 44. Ribbons of superparamagnetic colloids in magnetic field
 The European Physical Journal E
39, 47
 (2016)
 Show Abstract
 
 45. Statics and dynamics of magnetocapillary bonds
 Phys. Rev. E 
93, 053117
 (2016)
 Show Abstract
 
 46. Effect of relative air humidity on the flowability of lactose powders
 Journal of Drug Delivery Science and Technology
35, 207
 (2016)
 Show Abstract
 
 47. Magnetoelastic instability in soft thin films
 The European Physical Journal E
40, 29
 (2017)
 Show Abstract
 
 48. Relating Brownian motion to diffusion with superparamagnetic colloids
 American Journal of Physics 
85, 265
 (2017)
 Show Abstract
 
 49. Frustrated crystallization of a monolayer of magnetized beads under geometrical confinement
 Phys. Rev. E 
95, 062120
 (2017)
 Show Abstract
 
 50. Self-assembly processes of superparamagnetic colloids in a quasi-two-dimensional system
 Phys. Rev. E
96, 012608
 (2017)
 Show Abstract
 
 51. Superparamagnetic colloids in viscous fluids
 Scientific Reports
7, 7778
 (2017)
 Show Abstract
 
 52. Self-assembly of smart mesoscopic objects
 The European Physical Journal E
40, 108
 (2017)
 Show Abstract
 
 53. Discharge of repulsive grains from a silo: experiments and simulations
 EPJ Web of Conferences
140, 03089
 (2017)
 Show Abstract
 
 54. Combined effect of moisture and electrostatic charges on powder flow
 EPJ Web of Conferences
140, 13009
 (2017)
 Show Abstract
 
 55. Transitional bulk-solutal Marangoni instability in sessile drops
 Phys. Rev. E 
98, 062609
 (2018)
 Show Abstract
 
 56. Remote-controlled deposit of superparamagnetic colloidal droplets
 Phys. Rev. E 
98, 062608
 (2018)
 Show Abstract
 
 57. Decompaction of wet granular materials under freeze-thaw cycling
 Phys. Rev. E 
99, 012901
 (2019)
 Show Abstract
 
 58. From jamming to fast compaction dynamics in granular binary mixtures
 Scientific Reports
9, 7281
 (2019)
 Show Abstract
 
 59. Tribo-electrification of pharmaceutical powder blends
 Particulate Science and Technology
37, 1020
 (2019)
 Show Abstract
 
 60. How to gain a full understanding of powder flow properties, and the benefits of doing so
 ONdrugDelivery
102, 42
 (2019)
 Show Abstract
 
 61. Influence of mesoporous silica on powder flow and electrostatic properties on short and long term
 Journal of Drug Delivery Science and Technology
53, 101192
 (2019)
 Show Abstract
 
 62. Combined effects of Marangoni, sedimentation and coffee-ring flows on evaporative deposits of superparamagnetic colloids
 Colloid and Interface Science Communications
32, 100198
 (2019)
 Show Abstract
 
 63. Effect of volume fraction on chains of superparamagnetic colloids at equilibrium
 European Physical Journal E
42, 123
 (2019)
 Show Abstract
 
 
 |